Zinc oxide (ZnO) nanoparticles with different sizes and shapes were prepared by a grinding method. Phase identification was carried out by XRD, the results showed that all samples exhibited a wurtzite structure. The particle shapes were determined by SEM. A spherical structure changed to a flower shape when the OH- concentration increased. The optical band gap was evaluated by measurements of the optical absorption with a UV-Vis spectrophotometer. The optical band gap was dependent strongly on the defect concentration in the ZnO. In this study, the presence of the flower-like structure gave rise to a reduction of the optical band gap due to the increase of oxygen vacancies that could be confirmed by the EPR measurements.
Keywords: Grinding method, ZnO, Optical properties, Defects, EPR.